A supercontinuum white laser with ultrabroad bandwidth, intense pulse energy, and high spectral flatness can be accomplished via synergic action of third-order nonlinearity (3rd-NL) and second-order nonlinearity. In this work, we employ an intense Ti:sapphire femtosecond laser with a pulse duration of 50 fs and pulse energy up to 4 mJ to ignite the supercontinuum white laser. Remarkably, we use water instead of the usual solid materials as the 3rd-NL medium exhibiting both strong self-phase modulation and stimulated Raman scattering effect to create a supercontinuum laser with significantly broadened bandwidth and avoid laser damage and destruction. Then the supercontinuum laser is injected into a water-embedded chirped periodically poled lithium niobate crystal that enables broadband and high-efficiency second-harmonic generation. The output white laser has a 10 dB bandwidth encompassing 413 to 907 nm, more than one octave, and a pulse energy of 0.6 mJ. This methodology would open up an efficient route to creating a long-lived, high-stability, and inexpensive white laser with intense pulse energy, high spectral flatness, and ultrabroad bandwidth for application to various areas of basic science and high technology.

We demonstrate an ultra-broadband high temporal contrast infrared laser source based on cascaded optical parametric amplification, hollow-core fiber (HCF) and second harmonic generation processes. In this setup, the spectrum of an approximately 1.8 μm laser pulse has near 1 μm full bandwidth by employing an argon gas-filled HCF. Subsequently, after frequency doubling with cascaded crystals and dispersion compensation by a fused silica wedge pair, 9.6 fs (~3 cycles) and 150 μJ pulses centered at 910 nm with full bandwidth of over 300 nm can be generated. The energy stability of the output laser pulse is excellent with 0.8% (root mean square) over 20 min, and the temporal contrast is >10¹² at –10 ps before the main pulse. The excellent temporal and spatial characteristics and stability make this laser able to be used as a good seed source for ultra-intense and ultrafast laser systems.

Temporal contrast directly affects the interaction between ultraintense and ultrashort pulse lasers with matter. Seed laser sources with broad bandwidth and high temporal contrast are significant for overall temporal contrast enhancement. The technique of cascaded nonlinear processes with optical parametric amplification and second-harmonic generation is demonstrated for high temporal contrast seed source generation. Within 40 ps before the main pulse, the temporal contrast reaches over 10¹¹. The pulse energy and duration of the high-contrast pulse are 112 μJ and 70 fs, respectively. Considering its high beam quality and stability, this laser source can serve as a high-quality seed for Nd:glass-based ultraintense and ultrashort pulse laser facilities.

Infrared femtosecond optical vortices open up many new research fields, such as optical micro–nano manipulation, time-resolved nonlocal spectroscopy in solids, vortex secondary radiation and particle generations. In this article, we demonstrate a femtosecond optical vortex laser system based on a two-stage optical parametric amplifier. In our experiment, 1.45 μm vortex signal pulses with energy of 190 μJ and 1.8 μm vortex idler pulses with energy of 158 μJ have been obtained, and the pulse durations are 51 and 48 fs, respectively. Both the energy fluctuations of the signal and idler pulses are less than 0.5% (root mean square), and the spectral fluctuations are less than 1.5% within 1 hour. This type of highly stable femtosecond optical vortex laser has a wide range of applications for vortex strong-field physics.

We demonstrate the simultaneous temporal contrast improvement and pulse compression of a Yb-doped femtosecond laser via nonlinear elliptical polarization rotation in a solid state multi-pass cell. The temporal contrast is improved to 10⁹, while the pulse is shortened from 181 to 36 fs, corresponding to a compression factor of 5. The output beam features excellent beam quality with M² values of 1.18 × 1.16. The total efficiency of the contrast enhancement system exceeds 50%. This technique will have wide applications in high temporal contrast ultra-intense femtosecond lasers.